Journal
PHYSICAL REVIEW LETTERS
Volume 105, Issue 17, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.105.176601
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Funding
- BMBF [03SF0328]
- RCUK [GR/S85726]
- EPSRC [EP/C542398]
- Engineering and Physical Sciences Research Council [EP/C542398/1] Funding Source: researchfish
- EPSRC [EP/C542398/1] Funding Source: UKRI
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We report the observation of a spin-dependent dark transport current, exhibiting spin coherence at room temperature, in a pi-conjugated polymer-fullerene blend using pulsed electrically detected magnetic resonance. The resonance at g = 2.0028(3) is due to polarons in the polymer, and exhibits spin locking at high microwave fields. The presence of an excess of fullerene, and the operating voltage (1 V) used, suppresses negative polaron formation in the polymer. It is concluded that spin-dependent transport is due to the formation of positive bipolarons.
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