Journal
PHYSICAL REVIEW LETTERS
Volume 105, Issue 20, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.105.203201
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Funding
- Agence Nationale de la Recherche [ANR-BLAN-2006-0247]
- Conseil Regional d'Aquitaine [2007.1221]
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We report combined studies on the prototypical S(D-1(2)) + H-2 insertion reaction. Kinetics and crossed-beam experiments are performed in experimental conditions approaching the cold energy regime, yielding absolute rate coefficients down to 5.8 K and relative integral cross sections to collision energies as low as 0.68 meV. They are supported by quantum calculations on a potential energy surface treating long-range interactions accurately. All results are consistent and the excitation function behavior is explained in terms of the cumulative contribution of various partial waves.
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