Journal
PHYSICAL REVIEW LETTERS
Volume 105, Issue 20, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.105.203001
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- Japan Society for the Promotion of Science
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We report on the direct conversion of laser-cooled K-41 and Rb-87 atoms into ultracold (KRb)-K-41-Rb-87 molecules in the rovibrational ground state via photoassociation followed by stimulated Raman adiabatic passage. High-resolution spectroscopy based on the coherent transfer revealed the hyperfine structure of weakly bound molecules in an unexplored region. Our results show that a rovibrationally pure sample of ultracold ground-state molecules is achieved via the all-optical association of laser-cooled atoms, opening possibilities to coherently manipulate a wide variety of molecules.
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