Journal
PHYSICAL REVIEW LETTERS
Volume 102, Issue 8, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.102.086809
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Optical pump-probe spectroscopy with 7-fs pump pulses and a probe spectrum wider than 0.7 eV reveals the ultrafast carrier dynamics in freestanding thin graphite films. We discern for the first time a rapid intraband carrier equilibration within 30 fs, leaving the system with separated electron and hole chemical potentials. Phonon-mediated intraband cooling of electrons and holes occurs on a 100 fs time scale. The kinetics are in agreement with simulations based on Boltzmann equations.
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