Observation of a Soft Mode of Elastic Instability in Liquid Crystal Elastomers

In monodomain liquid crystal elastomers a symmetry-breaking locked-in anisotropy causes a semisoft elastic response characterized by a plateau in the stress-strain curve. We show by dynamic light scattering performed as a function of deformation that the relaxation rate of the nematic director fluctuations decreases with strain to a very small value at the onset of the soft elastic response, revealing the existence of a dynamic soft mode. The results are in complete agreement with the theory of semisoft elasticity and allow us to determine all the constants of the model.