4.8 Article

Percolation Model for Slow Dynamics in Glass-Forming Materials

Journal

PHYSICAL REVIEW LETTERS
Volume 102, Issue 1, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.102.015702

Keywords

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Funding

  1. NSF [CBET-0348175, DMR-0448838]
  2. Yale's Institute for Nanoscience and Quantum Engineering

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We identify a link between the glass transition and percolation of regions of mobility in configuration space. We find that many hallmarks of glassy dynamics, for example, stretched-exponential response functions and a diverging structural relaxation time, are consequences of the critical properties of mean-field percolation. Specific predictions of the percolation model include the range of possible stretching exponents 1/3 <=beta <= 1 and the functional dependence of the structural relaxation time tau(alpha) and exponent beta on temperature, density, and wave number.

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