Journal
PHYSICAL REVIEW LETTERS
Volume 100, Issue 9, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.100.093006
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Laser-aligned carbondisulfide (CS2) molecules are singly ionized by multiphoton absorption from intense, linearly polarized 25 fs laser pulses. The angular distribution of the photoelectrons exhibits a significant dependence on the angle between the polarizations of the aligning and ionizing laser fields. The widely used strong-field approximation predicts angular distributions in qualitative agreement with the experimental data but fails at a quantitative level.
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