Journal
PHYSICAL REVIEW LETTERS
Volume 101, Issue 25, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.101.253001
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Funding
- U. K. EPSRC [EP/ E000223/1]
- Engineering and Physical Sciences Research Council [EP/E000223/1] Funding Source: researchfish
- EPSRC [EP/E000223/1] Funding Source: UKRI
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An attosecond pump-probe scheme that combines the use of a free-electron laser pulse with an ultrashort pulse is applied in order to explore the ultrafast excitation dynamics in Ne. We describe the multielectron dynamics using a new nonperturbative time-dependent R-matrix theory. This theory enables the interaction of ultrashort light fields with multielectron atoms and atomic ions to be determined from first principles. By probing the emission of an inner 2s electron from Ne we are also able to study the bound state population dynamics during the free-electron laser pulse.
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