Journal
PHYSICAL REVIEW E
Volume 78, Issue 4, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevE.78.046711
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Funding
- Competence Center of Energy and Mobility (CCEM) of Switzerland
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A lattice Boltzmann model is developed to simulate finite-rate catalytic surface chemistry. Diffusive wall boundary conditions are established to account for catalytic reactions in multicomponent mixtures. Implementation of wall boundary conditions with chemical reactions is based on a general second-order accurate interpolation scheme. Results of lattice Boltzmann simulations for a four-component mixture with a global catalytic methane oxidation reaction in a straight channel are in excellent agreement with a finite volume Navier-Stokes solver in terms of both the flow field and species concentrations.
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