Journal
PHYSICAL REVIEW B
Volume 90, Issue 9, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.90.094116
Keywords
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Funding
- Air Force Office of Scientific Research [AF FA 9550-11-1-0073]
- Office of Naval Research [N00014-10-10525]
- Defense Advanced Research Projects Agency (DARPA) [N66001-11-1-4195]
- Army Research Office [W911NF-10-1-0482]
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We report laser-based direct measurements of the pyroelectric and electrocaloric effects of PbZr1-xTixO3 epitaxial layers as a function of temperature and electric field. By evaluating the differences between the total pyroelectric and electrocaloric coefficients, we determine the secondary contribution to the electrocaloric effect that is created by a combination of piezoelectric and elastocaloric effects. The secondary contribution to the electrocaloric coefficient has the opposite sign as the primary effect and therefore reduces the overall entropy change of PbZr1-xTixO3 in an electric field. The absolute magnitude of the secondary effect is comparable to the primary effect at elevated temperatures of approximate to 200 degrees C.
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