Journal
PHYSICAL REVIEW B
Volume 89, Issue 20, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.89.205122
Keywords
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Funding
- NSF [DMR-1066158, 0918970]
- ONR [N00014-11-1-0384, N000-14-12-1-1034]
- Ministry of Science and Technology of China [2011CB606405]
- National Natural Science Foundation of China [11174173]
- China Scholarship Council
- MRI [0722625]
- MRI-R2 [0959124]
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First-principles calculations are performed to predict structural, electric, magnetic, and magnetoelectric properties of hexagonal rare-earth ferrites (RFeO3) under chemical and hydrostatic pressures. Decreasing the rare-earth ionic radius has two dramatic consequences: (i) an enhancement of the electrical polarization by a factor of 60% and (ii) a magnetic transition, which renders the systems (weakly) ferromagnetic. Moreover and unlike conventional ferroelectrics, the electrical polarization strengthens as a hydrostatic pressure is applied and increases in magnitude in any hexagonal rare-earth ferrites. Finally, applying a hydrostatic pressure in RFeO3 having small or intermediate rare-earth ionic radius results in the sudden disappearance of a weak magnetization and of the linear magnetoelectric effect above some critical pressure. Origins of these striking effects are revealed.
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