4.6 Article

Mechanisms for sub-gap optical conductivity in Herbertsmithite

Journal

PHYSICAL REVIEW B
Volume 87, Issue 24, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.87.245106

Keywords

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Funding

  1. NSF [DMR 1104498, DMR-1005434]
  2. National Science Foundation [NSF PHY11-25915]
  3. Simons Foundation [229736]
  4. Direct For Mathematical & Physical Scien
  5. Division Of Materials Research [1104498] Funding Source: National Science Foundation

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Recent terahertz conductivity measurements observed low-power-law frequency dependence of optical conduction within the Mott gap of the kagome lattice spin-liquid candidate Herbertsmithite. We investigate mechanisms for this observed sub-gap conductivity for two possible scenarios in which the ground state is described by (1) a U(1) Dirac spin liquid with emergent fermionic spinons or (2) a nearly critical Z(2) spin liquid in the vicinity of a continuous quantum phase transition to magnetic order. We identify new mechanisms for optical absorption via magnetoelastic effects and spin-orbit coupling. In addition, for the Dirac spin liquid scenario, we establish an explicit microscopic origin for previously proposed absorption mechanisms based on slave-particle effective field theory descriptions.

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