4.6 Article

Nuclear magnetic resonance studies of pseudospin fluctuations in URu2Si2

Journal

PHYSICAL REVIEW B
Volume 88, Issue 9, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.88.094436

Keywords

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Funding

  1. UC Lab Research Fee Program
  2. NNSA through US DOE [DE-FG52-09NA29464]
  3. Center for Integrated Nanotechnologies, an Office of Science User Facility
  4. US DOE Office of Science [DE-AC52-06NA25396]
  5. Nordita
  6. Alexander von Humboldt foundation
  7. US Department of Energy [DE-FG02-04ER46105]
  8. Direct For Mathematical & Physical Scien
  9. Division Of Materials Research [1005393] Funding Source: National Science Foundation

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We report Si-29 nuclear magnetic resonance measurements in single crystals and aligned powders of URu2Si2 in the hidden order and paramagnetic phases. The spin-lattice relaxation data reveal evidence of pseudospin fluctuations of U moments in the paramagnetic phase. We find evidence for partial suppression of the density of states below 30 K and analyze the data in terms of a two-component spin-fermion model. We propose that this behavior is a realization of a pseudogap between the hidden-order transition T-HO and 30 K. This behavior is then compared to other materials that demonstrate precursor fluctuations in a pseudogap regime above a ground state with long-range order.

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