Journal
PHYSICAL REVIEW B
Volume 85, Issue 5, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.85.052301
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We have studied a promising lithium-ion conductor, garnet-type cubic Li oxides, at various Li concentrations. The ab initio calculations performed on these materials revealed two distinct mechanisms of Li-ion transport, with very different energy barriers and a strong dependence on Li distribution. Our findings explain the origin of the vastly varying ionic conductivities at different Li concentrations and suggest possible principles to improve such materials for solid-state electrolyte applications.
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