4.6 Article

Resonance-hybrid states in a triple quantum dot

Journal

PHYSICAL REVIEW B
Volume 85, Issue 8, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.85.081301

Keywords

-

Funding

  1. JSPS [23740248, 19104007]
  2. MEXT [21102003]
  3. Project for Developing Innovation Systems (NanoQuine)
  4. Funding Program for World-Leading Innovative R&D on Science and Technology (FIRST)
  5. Harvard University
  6. Grants-in-Aid for Scientific Research [23740248, 19104007, 21102003] Funding Source: KAKEN

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Delocalization by resonance between contributing structures explains the enhanced stability of resonance-hybrid molecules. Here we report the realization of resonance-hybrid states in a few-electron triple quantum dot (TQD) obseved by excitation spectroscopy. The stabilization of the resonance-hybrid state and the bond between contributing states are achieved through access to the intermediate states with double occupancy of the dots. This explains why the energy of the hybridized singlet state is significantly lower than that of the triplet state. The properties of the three-electron doublet states can also be understood with the resonance-hybrid picture and geometrical phase. As well as for fundamental TQD physics, our results are useful for the investigation of materials such as quantum dot arrays, quantum information processors, and chemical reaction and quantum simulators.

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