4.6 Article

Magnetophonon resonance in graphite: High-field Raman measurements and electron-phonon coupling contributions

Journal

PHYSICAL REVIEW B
Volume 85, Issue 12, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.85.121403

Keywords

-

Funding

  1. NHMFL [UCGP-5068]
  2. DOE/BES [DE-FG02-07ER46451, DE-FG02-06ER46308]
  3. Robert A. Welch Foundation [C-1509]
  4. Texas NHARP [01889]
  5. A. P. Sloan Foundation
  6. EPSRC [GR/S97613/01, EP/E500935/1]
  7. ERC
  8. EU
  9. Royal Society
  10. NSF [DMR-0654118]
  11. State of Florida
  12. Engineering and Physical Sciences Research Council [EP/E500935/1, GR/S97613/01] Funding Source: researchfish
  13. EPSRC [EP/E500935/1] Funding Source: UKRI
  14. Direct For Mathematical & Physical Scien
  15. Division Of Materials Research [1006663] Funding Source: National Science Foundation

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We perform Raman scattering experiments on natural graphite in magnetic fields up to 45 T, observing a series of peaks due to interband electronic excitations over a much broader magnetic field range than previously reported. We also explore electron-phonon coupling in graphite via magnetophonon resonances. The Raman G peak shifts and splits as a function of magnetic field, due to the magnetically tuned coupling of the E-2g optical phonons with the K- and H-point inter-Landau-level excitations. The analysis of the observed anticrossing behavior allows us to determine the electron-phonon coupling for both K- and H-point carriers. In the highest field range (> 35 T) the G peak narrows due to suppression of electron-phonon interaction.

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