4.6 Article

Resonance energy transfer near metal nanostructures mediated by surface plasmons

Journal

PHYSICAL REVIEW B
Volume 83, Issue 8, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.83.085427

Keywords

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Funding

  1. NSF [DMR-0906945, HRD-0833178]
  2. EPSCOR program
  3. Division Of Human Resource Development
  4. Direct For Education and Human Resources [833178] Funding Source: National Science Foundation
  5. EPSCoR
  6. Office Of The Director [903787] Funding Source: National Science Foundation

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We develop a unified theory of plasmon-assisted resonance energy transfer (RET) between molecules near a metal nanostructure that maintains energy balance between transfer, dissipation, and radiation. We show that in a wide range of parameters, including in the near field, RET is dominated by plasmon-enhanced radiative transfer (PERT) rather than by a nonradiative transfer mechanism. Our numerical calculations performed for molecules near the Ag nanoparticle indicate that RET magnitude is highly sensitive to molecules' positions.

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