4.6 Article

Charge transfer statistics of a molecular quantum dot with strong electron-phonon interaction

Journal

PHYSICAL REVIEW B
Volume 83, Issue 8, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.83.085401

Keywords

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Funding

  1. DFG [KO 2235/3]
  2. Kompetenznetz Funktionelle Nanostrukturen III of the Baden-Wurttemberg Stiftung (Germany)
  3. Swiss NSF
  4. HGSFP of the University of Heidelberg
  5. CQD of the University of Heidelberg

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We analyze the nonequilibrium transport properties of a quantum dot with a harmonic degree of freedom (Holstein phonon) coupled to metallic leads, and derive its full counting statistics. By using the Lang-Firsov (polaron) transformation, we construct a diagrammatic scheme to calculate the cumulant generating function. The electron-phonon interaction is taken into account exactly, and the employed approximation represents a summation of a diagram subset with respect to the tunneling amplitude. By comparison to Monte Carlo data, the formalism is shown to capture the basic properties of the strong-coupling regime.

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