4.6 Article

Magnetic nanoscale laminates with tunable exchange coupling from first principles

Journal

PHYSICAL REVIEW B
Volume 84, Issue 22, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.84.220403

Keywords

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Funding

  1. European Research Council under the European Community [258509]
  2. Centre in Nanoscience and Technology (CeNano)
  3. Swedish Research Council (VR)
  4. Swedish e-Science Research Centre (SeRC)
  5. research center Advanced Functional Materials (AFM)
  6. Goran Gustafsson Foundation for Research in Natural Sciences and Medicine

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The M(n+1)AX(n) (MAX) phases are nanolaminated compounds with a unique combination of metallic and ceramic properties, not yet including magnetism. We carry out a systematic theoretical study of potential magnetic MAX phases and predict the existence of stable magnetic (Cr1-xMnx)(2)AlC alloys. We show that in this system ferromagnetically ordered Mn layers are exchange coupled via nearly nonmagnetic Cr layers, forming an inherent structure of atomic-thin magnetic multilayers, and that the degree of disorder between Cr and Mn in the alloy can be used to tune the sign and magnitude of the coupling.

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