Journal
PHYSICAL REVIEW B
Volume 84, Issue 2, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.84.024422
Keywords
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Funding
- MICINN (Spain) [FIS2009-08744]
- European Research Council [STEMOX 239739]
- US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division
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Electric-field controlled exchange bias in a heterostructure composed of the ferromagnetic manganite La0.7Sr0.3MO3 and the ferroelectric antiferromagnetic BiFeO3 has recently been demonstrated experimentally. By means of a model Hamiltonian, we provide a possible explanation for the origin of this magnetoelectric coupling. We find, in agreement with experimental results, a net ferromagnetic moment at the BiFeO3 interface. The induced ferromagnetic moment is the result of the competition between the e(g)-electron double exchange and the t(2g)-spin antiferromagnetic superexchange that dominates in bulk BiFeO3. The balance of these simultaneous ferromagnetic and antiferromagnetic tendencies is strongly affected by the interfacial electronic charge density, which, in turn, can be controlled by the BiFeO3 ferroelectric polarization.
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