Journal
PHYSICAL REVIEW B
Volume 82, Issue 8, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.82.081410
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Funding
- NSF [CHE 07 17518]
- Grants-in-Aid for Scientific Research [22750039] Funding Source: KAKEN
- Engineering and Physical Sciences Research Council [EP/G035695/1] Funding Source: researchfish
- EPSRC [EP/G035695/1] Funding Source: UKRI
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We report an inelastic neutron-scattering (INS) investigation of coupled quantum translation and rotation of hydrogen molecules trapped inside the closed isotropic cages of C-60. The low-lying states that characterize the translation-rotation manifold of the hydrogen molecules are accurately determined in our study of the INS peak energies. A comparison between the spectra of H-2 and HD isotopomers provides quantitative insight into the coupling between rotational and translational angular momentum with HD exhibiting the strongest effects due to mixing of the rotational eigenstates.
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