Journal
PHYSICAL REVIEW B
Volume 82, Issue 23, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.82.235431
Keywords
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Funding
- German Science Foundation (DFG) [560398]
- European Research Council (ERC) [240556]
- European Commission [220505]
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We analyze the effect of an electrostatic surface charge on the angular nonlinear light scattering pattern from spherical particles in solution. An electrostatic field near a charged interface leads to a bulk-allowed third-order process, the strength of which is proportional to the electrostatic surface potential. The commonly isotropic nature of the bulk leads to a fixed angular scattering pattern with fixed intensity ratios between polarizations. We show that second-and third-order scattering effects are separable due to their different angular radiation patterns. Furthermore, nonlinear light scattering from a third-order contribution is strongest in the ppp polarization combination.
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