Journal
PHYSICAL REVIEW B
Volume 82, Issue 12, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.82.125427
Keywords
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Funding
- Australian Research Council
- Israeli Academy of Science and Arts
- Technion Fund for promotion of research
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The effect of surface termination on C 1s core-level bulk excitons found near the surface in single-crystal diamond is reported. By simultaneously recording bulk (total electron yield) and surface (partial electron yield) near-edge x-ray absorption fine-structure (NEXAFS) spectra with a range of single-crystal surface terminations, variable bulk exciton energy blueshifts and linewidth broadening were observed, most notably in the reconstructed single-crystal diamond. Investigation of polycrystalline diamond and ultrananocrystalline diamond films, using the same technique, allowed for a comparison between the reconstructed single-crystal diamond surface and nanodiamond bulk excitons. These findings suggest that surface-related effects can be misinterpreted as quantum confinement in some nanodiamond NEXAFS studies. Band bending is suggested as a possible contributor to these results.
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