Journal
PHYSICAL REVIEW B
Volume 80, Issue 12, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.80.121403
Keywords
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Funding
- Nanoscale Science and Engineering Initiative of the NSF [CHE0117752, ECS-05-07111]
- New York State Office of Science, Technology, and Academic Research (NYSTAR)
- Chemical Sciences, Geosciences, and Biosciences Division
- Office of Basic Sciences
- Office of Science, U. S. Department of Energy the Office of Basic Energy Sciences
- Alexander-von-Humboldt Foundation
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Time-resolved Raman spectroscopy has been applied to probe the anharmonic coupling and electron-phonon interaction of optical phonons in graphite. From the decay of the transient anti-Stokes scattering of the G-mode following ultrafast excitation, we measured a lifetime of 2.2 +/- 0.1 ps for zone-center optical phonons. We also observed a transient stiffening of G-mode phonons, an effect attributed to the reduction of the electron-phonon coupling for high electronic temperatures.
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