Journal
PHYSICAL REVIEW A
Volume 82, Issue 1, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevA.82.011403
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Funding
- Stifterverband fur die Deutsche Wissenschaft
- Fonds der Chemischen Industrie
- Deutsche Forschungsgemeinschaft [Sa 936/2]
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The alignment dependence of the ionization behavior of H-2 exposed to intense ultrashort laser pulses is investigated on the basis of solutions of the full time-dependent Schrodinger equation within the fixed-nuclei and dipole approximation. The total ionization yields as well as the energy-resolved electron spectra have been calculated for a parallel and a perpendicular orientation of the molecular axis with respect to the polarization axis of linear polarized laser pulses. For most, but not all considered laser peak intensities, the parallel aligned molecules are easier to ionize. Furthermore, it is shown that the velocity formulation of the strong-field approximation predicts a simple interference pattern for the ratio of the energy-resolved electron spectra obtained for the two orientations, but this is not confirmed by the full ab initio results.
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