Journal
PHYSICAL REVIEW A
Volume 82, Issue 1, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevA.82.013408
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Funding
- Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, US Department of Energy
- National Science Foundation [CHE-0822646]
- DFG
- Cluster of Excellence: Munich Center for Advanced Photonics
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [0822646] Funding Source: National Science Foundation
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We have tracked nuclear wave-packet dynamics in doubly charged states of molecular oxygen using few-cycle infrared laser pulses. Bound and dissociating wave packets were launched and subsequently probed via a pair of 8-fs pulses of 790 nm radiation. Ionic fragments from the dissociating molecules were monitored by velocity-map imaging. Pronounced oscillations in the delay-dependent kinetic energy release spectra were observed. The occurrence of vibrational revivals permits us to identify the potential curves of the O-2 dication which are most relevant to the molecular dynamics. These studies show the accessibility to the dynamics of such higher-charged molecules.
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