Journal
PHYSICAL REVIEW A
Volume 81, Issue 5, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevA.81.051402
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Funding
- DFG [JI 110/2-2]
- MICINN [FIS2007-60064]
- NSF [PHY-0652519]
- Division Of Physics
- Direct For Mathematical & Physical Scien [0969299, GRANTS:14052687] Funding Source: National Science Foundation
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We used a split-mirror setup attached to a reaction microscope at the free-electron laser in Hamburg (FLASH) to perform an XUV-pump-XUV-probe experiment by tracing the ultrafast nuclear wave-packet motion in the D-2(+)(1s sigma(g)) with 10 fs time resolution. Comparison with time-dependent calculations shows excellent agreement with the measured vibrational period of 22 +/- 4 fs in D-2(+), points to the importance of accurately knowing the internuclear distance-dependent ionization probability, and paves the way to control sequential and nonsequential two-photon double-ionization contributions.
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