Journal
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
Volume 15, Issue 38, Pages 15833-15839Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cp53428f
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Funding
- National Science Foundation [DMR-08-19762]
- Advanced Research Projects Agency-Energy (ARPA-E), US Department of Energy [DE-AR0000065]
- Joint Center for Energy Storage Research (JCESR)
- US Department of Energy
- agency of the United States Government. Neither the United States Government
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An aqueous Li-ion flow cell using suspension-based flow electrodes based on the LiTi2(PO4)(3)-LiFePO4 couple is demonstrated. Unlike conventional flow batteries, the semi-solid approach utilizes fluid electrodes that are electronically conductive. A model of simultaneous advection and electrochemical transport is developed and used to separate flow-induced losses from those due to underlying side reactions. The importance of plug flow to achieving high energy efficiency in flow batteries utilizing highly non-Newtonian flow electrodes is emphasized.
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