4.6 Article

Sorption enhanced CO2 methanation

Journal

PHYSICAL CHEMISTRY CHEMICAL PHYSICS
Volume 15, Issue 24, Pages 9620-9625

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cp51408k

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Funding

  1. CCEM
  2. Swisselectric research through the HyTech project

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The transformation from the fatuous consumption of fossil energy towards a sustainable energy circle is most easily marketable by not changing the underlying energy carrier but generating it from renewable energy. Hydrocarbons can be principally produced from renewable hydrogen and carbon dioxide collected by biomass. However, research is needed to increase the energetic and economic efficiency of the process. We demonstrate the enhancement of CO2 methanation by sorption enhanced catalysis. The preparation and catalytic activity of sorption catalysts based on Ni particles in zeolites is reported. The functioning of the sorption catalysis is discussed together with the determination of the reaction mechanism, providing implications for new ways in catalysis.

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