Journal
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
Volume 13, Issue 18, Pages 8127-8130Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0cp02705g
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Funding
- Agence Nationale de la Recherche [ANR-BLAN-2006-0247]
- Conseil Regional d'Aquitaine [2007.1221]
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The integral cross section of the S(D-1(2)) + H-2(j = 0) -> SH + H reaction has been measured for the first time at collision energies from 0.820 down to 0.078 kJ mol(-1) in a high-resolution crossed beam experiment. The excitation function obtained exhibits a non-monotonic variation with collision energy and compares well with the results of high-level quantum calculations. In particular, the structures observed in the lower energy part, where only a few partial waves contribute, can be described in terms of the sequential opening of individual channels, consistent with the theoretical calculations.
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