Journal
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
Volume 11, Issue 37, Pages 8149-8155Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/b905702a
Keywords
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Funding
- 'Programme National Physique et Chimie du Milieu Interstellaire'
- Agence Nationale de la Recherche [ANR-JC08_311018]
- European Union [PERG03-GA-2008-230805]
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The kinetics of the N(S-4 degrees) + NO(X-2 Pi) reaction have been studied in a continuous supersonic flow reactor over the range 48 K <= T <= 211 K. Nitrogen atoms were produced by microwave discharge upstream of the Laval nozzle and were probed in the vacuum ultraviolet by resonance fluorescence. The reaction has been found to exhibit a small negative temperature dependence, with a rate coefficient decreasing from (5.8 +/- 0.3) x 10(-11) cm(3) molecule(-1) s(-1) at 48 K to (3.3 +/- 0.2) x 10(-11) cm(3) molecule(-1) s(-1) at 211 K with the statistical uncertainties cited at the level of a single standard deviation from the mean.
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