Journal
PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES
Volume 370, Issue 1972, Pages 3709-3727Publisher
ROYAL SOC
DOI: 10.1098/rsta.2011.0219
Keywords
carotenoids; nonlinear optical spectroscopy; diagrammatic representations; four-wave mixing; impulsive Raman
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Funding
- National Science Foundation [CHE-1058791]
- National Institutes of Health [GM-59230]
- Defense Advanced Research Projects Agency [UOFT-49606]
- Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Science, US Department of Energy [DE-FG02-04ER15571]
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Two types of diagrammatic approaches for the design and simulation of nonlinear optical experiments (closed-time path loops based on the wave function and double-sided Feynman diagrams for the density matrix) are presented and compared. We give guidelines for the assignment of relevant pathways and provide rules for the interpretation of existing nonlinear experiments in carotenoids.
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