Journal
ORGANOMETALLICS
Volume 28, Issue 24, Pages 6847-6854Publisher
AMER CHEMICAL SOC
DOI: 10.1021/om900275j
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Funding
- Hong Kong Research Grant Council [HKUST 601306, HKUST 601505, HKUI/CRF/08]
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The catalytic activity of a series of ruthenium complexes for C-H amination reactions of organic 9 which promotes C-H azides was investigated. The most active catalyst was found to be RuCl3, amination reactions of ortho-aryl phenylazides, 1-azido-2-arylvinylazides, and 1-azido-1,3-butadienes to give carbazoles, indoles, and pyrroles, respectively. Both computational and experimental results support that a two-step process involving formal electrocyclization is involved in the catalytic reaction.
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