Journal
ORGANIC LETTERS
Volume 16, Issue 13, Pages 3584-3587Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol501584d
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Funding
- 973 Program [2011CB808600, 2012CB725302]
- National Natural Science Foundation of China [21390400, 21025206, 21272180, 21302148]
- Research Fund for the Doctoral Program of Higher Education of China [20120141130002]
- Program for Changjiang Scholars and Innovative Research Team in University [IRT1030]
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By combining catalytic nucleophilic enamine activation with Pd-catalyzed C H activation of allylarenes, the first oxidative allylic alkylation of unactivated ketones was achieved. Mechanistically, the Pd-catalyzed allylic C H activation and proline-catalyzed ketone nucleophilic activation worked synergistically for the oxidative cross-coupling between allylarenes and unactivated ketones.
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