Journal
ORGANIC LETTERS
Volume 16, Issue 12, Pages 3176-3179Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol500663b
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Funding
- National Science Council of Taiwan [NSC 101-2113-M-002-009-MY3, 102-2221-E-259-025]
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A new synthetic strategy for indolo[2,3-b]carbazole via a double-intramolecular Buchwald-Hartwig reaction has been established. The N-alkylated indolo[2,3-b]carbazole then was adopted as the geometry-fixed core for the synthesis of a new molecule (ICZDTA) bearing two bithiophene pi-bridged 2-cyanoacrylic acid groups as the bidentate anchor. The bidentate anchoring together with efficient HOMO (indolo[2,3-b]carbazole) -> LUMO (TiO2 nanocluster) electron transfer leads to the successful development of ICZDTA-based DSSC with a power conversion efficiency of 6.02%.
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