Journal
ORGANIC LETTERS
Volume 16, Issue 10, Pages 2575-2577Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol500811u
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The flavor menthon (isomeric mixture of (-)-menthon and (+)-isomenthon) was obtained in good yields and selectivities by a solventless ruthenium catalyzed isomerization of the homoallylic alcohol (-)-isopulegol. In contrast to most previous assumptions on such isomerization reactions, this reaction follows an intermolecular pathway, with menthol and pulegon being the central intermediates in this transformation.
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