Journal
ORGANIC LETTERS
Volume 16, Issue 23, Pages 6196-6199Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol503121q
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Funding
- Spanish MINECO [SAF2013-41943-R]
- ERDF
- European Research Council [340055]
- Xunta de Galicia [GRC2013-041]
- European Research Council (ERC) [340055] Funding Source: European Research Council (ERC)
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alpha,beta-Unsaturated N,N-dialkyl hydrazones undergo a mild [2 + 2] cycloaddition to allenamides when treated with a suitable gold catalyst. The method, which represents the first application of N,N-dialkyl hydrazones in gold catalysis, is compatible with a wide variety of substituents at the alkenyl moiety of the hydrazone component, proceeds with excellent levels of regio- and diastereoselectivity, and provides densely substituted cyclobutanes with good to excellent yields.
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