Journal
ORGANIC LETTERS
Volume 16, Issue 18, Pages 4884-4887Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol5023933
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Funding
- NSFC [21272276]
- SKLNM [JKGZ201110, ZZJQ201306]
- Ministry of Education of China [PSCIRT-1193]
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A solvent-controlled switchable C-H alkenylation of 4-aryl-1H-pyrrole-3-carboxylates via a Pd(OAc)(2) catalyzed oxidative Heck reaction was first realized. The corresponding C2 and C5 alkenylation products were obtained in good yields with high regioselectivities, respectively. The selective C5-alkenylation was successfully applied to the total synthesis of (+/-)-rhazinilam.
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