Journal
ORGANIC LETTERS
Volume 16, Issue 20, Pages 5486-5489Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol502766q
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Funding
- National Institutes of Health [GM57O14]
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Advances in hydroarylation have been achieved by the development of a one-pot regioselective allene hydrosilylation/Pd(0)catalyzed cross-coupling protocol. The regioselectivity is primarily governed by N-heterocyclic carbene(NHC)ligand identity in the hydrosilylation step and is preserved in the subsequent cross-coupling reaction. This methodology affords streamlined access to functionalized 1,1-disubstituted alkenes with excellent regiocontrol.
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