Journal
ORGANIC LETTERS
Volume 16, Issue 24, Pages 6440-6443Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol503275w
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Funding
- NSF [CHM-0709061]
- NDSU
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Enantioselective conjugate addition of malononitrile to pyrazolidinone-derived enoates proceeds in excellent yields and high enantioselectivities. A comparison of fluxional substituents with and without a Bronsted basic site and their impact on selectivity is detailed. Molecular sieves as an additive were found to be essential to achieve high enantioselectivity.
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