Journal
ORGANIC LETTERS
Volume 16, Issue 11, Pages 2974-2977Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol501115m
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Funding
- JSPS [25220802]
- Grants-in-Aid for Scientific Research [26810021, 25620031] Funding Source: KAKEN
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FeCl3-mediated oxidative fusion of meso-linked dibenzo[a,g]corannulene porphyrin dyads 6M afforded fused porphyrins 7M bearing a five-membered ring connection, but similar oxidation of beta-linked dyads 9M provided fused porphyrins 10M bearing a six-membered ring connection, both in a regiospecific manner. While fused dyads 10M exhibit modestly red-shifted absorption and fluorescence profiles, fused dyads 7M display characteristically red-shifted absorption bands reflecting antiaromatic dehydropurpurin electronic networks.
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