Journal
ORGANIC LETTERS
Volume 16, Issue 8, Pages 2204-2207Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol5007218
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- UGC
- IIT Kanpur, India
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An unprecedented and domino synthetic strategy for the synthesis of highly functionalized carbocyclic beta-enaminoesters bearing an all-carbon quaternary center via Yb(OTf)(3)-catalyzed ring-opening cyclization/decarboxylative tautomerization of donor acceptor cyclopropanes with 2-alkyl malononitriles in excellent yields is described: The products are obtained as a single diastereomer in most cases where the nitrile and aryl groups are aligning in a cis orientation across the ring.
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