Journal
ORGANIC LETTERS
Volume 15, Issue 19, Pages 4960-4963Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol402201c
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Funding
- Indian Institute of Technology Madras through New Faculty Scheme
- Council of Scientific & Industrial Research (CSIR)
- CSIR
- IITM
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A rhodium-catalyzed cyanation of chelation assisted C-H bonds is described employing N-cyano-N-phenyl-p-methylbenzenesulfonamide as an efficient cyanating reagent. The present method allowed the synthesis of various benzonitirle derivatives in good to excellent yield. A number of chelating groups are also effective in the present cyanation of C-H bonds. In addition, the developed methodology was applied in the formal synthesis of the isoquinoline alkaloid, menisporphine.
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