Journal
ORGANIC LETTERS
Volume 15, Issue 8, Pages 1990-1993Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol400659p
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- Institute for Basic Science (IBS)
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Cyanation of aryl-, diaryldimethyl-, and styrylsilanes was developed for the first time under copper-mediated oxidative conditions using ammonium iodide and DMF as the combined source of nitrogen and carbon atom of the introduced cyano unit, respectively. The reaction was observed to proceed in a two-step process: initial conversion of organosilanes to their iodo intermediates and then cyanation. This method has a broad substrate scope with high functional group tolerance.
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