Journal
ORGANIC LETTERS
Volume 15, Issue 23, Pages 5956-5959Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol402804t
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Funding
- National Natural Science Foundation of China [21362043, 21162040, 21302162]
- Government of Yunnan Province [2012FB170]
- State Key Laboratory of Elemento-organic Chemistry, Nankai University [201206]
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The complexes of various Rh precusors with ferrocenyl chiral ligand (R,S)-Cy2PF-PPh2 were found effective catalysts for the asymmetric hydroalkynylation reaction of norbornadiene derivatives. When RhCl3 center dot 3H(2)O was employed, good yields (up to 98%) and high enantioselectivities (up to >99.9% ee) could be obtained for the reactions of a broad scope of substrates.
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