Journal
ORGANIC LETTERS
Volume 15, Issue 7, Pages 1436-1439Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol4001262
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Funding
- MEXT
- IGER, NU
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A virtually salt-free and straightforward bimolecular assembly giving N-unsubstituted pyrroles through fully unmasked a-amino aldehydes, which was enabled by the dual effects of a catalytic ruthenium complex and an alkali metal base, is reported. Either solvent-free or acceptorless dehydrogenation facilitates high atom, step, and pot economy, which are otherwise difficult to achieve in multistep operations involving protection/deprotection.
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