Journal
ORGANIC LETTERS
Volume 15, Issue 24, Pages 6158-6161Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol403018x
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Funding
- MINECO of Spain [CTQ2012-37420-C02-01/BQU, CSD2010-00065]
- Catalan DIUE [2009SGR637]
- MICINN
- ICREA-Academia
- INNPLANTA Project [IPN-2011-0059-PCT-42000-ACT1]
- IOF
- [ERC-2009-StG-239910]
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Fast, efficient, and highly stereoselective epoxidation with H2O2 is reached by manganese coordination complexes with e-rich aminopyridine tetradentate ligands. It is shown that the electronic properties of these catalysts vary systematically with the stereoselectivity of the O-atom transfer event and exert fine control over the activation of hydrogen peroxide, reducing the amount of carboxylic acid co-catalyst necessary for efficient operation.
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