Journal
ORGANIC LETTERS
Volume 15, Issue 13, Pages 3226-3229Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol4011739
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Funding
- Fonds der chem. Industrie
- Merck
- NSERC for an Industrial Research Chair, the University of Toronto
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An asymmetric one-pot tandem Au/Rh-catalyzed synthesis of highly enantioenriched beta-disubstituted ketones starting from racemic propargyl alcohols is disclosed. The compatibility of the two metal complexes (Au/Rh) and their orthogonal ligand systems (NHC/diene) in this bimetallic catalytic system is investigated.
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