Journal
ORGANIC LETTERS
Volume 15, Issue 17, Pages 4362-4365Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol4018694
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Funding
- Indiana University
- American Chemical Society [PRF 52233-DNI1]
- NSF-CAREER [CHE-1254783]
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [1254783] Funding Source: National Science Foundation
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A new route to trisubstituted olefins through a palladium-catalyzed alkyne insertion/reduction reaction with unactivated alkyl iodides is reported. The reaction proceeds under mild conditions and tolerates a range of functional groups and substitution patterns. Preliminary mechanistic inquiry suggests that the transformation may proceed through a hybrid radical/organometallic pathway.
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