Journal
ORGANIC LETTERS
Volume 15, Issue 20, Pages 5338-5341Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol4025953
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Funding
- National Science Council
- Ministry of Education
- Center for Interdisciplinary Science (CIS) of the National Chiao Tung University, Taiwan
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A new strategy to synthesize 4,9- and 5,10-dialkylated alpha-aNDTs as well as 4,9- and 5,10-dialkylated beta-aNDTs is described. Four isomeric precursors with different dithienyl-ene-diyne arrangements undergo base-induced double 6 pi-cyclization to construct the central naphthalene cores, leading to the formation of the regiospecific products. These 2,7-distannylated dialkylated aNDT-based monomers can be used for Stille cross-coupling to produce promising conjugated materials for various optoelectronic applications.
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